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The Raleigh-based chain Port City Java, 701 North Carolina Ave SE, +1 202 544-7770, M-F 6:30AM-7PM, offers free WiFi. Otherwise, the two public libraries in the neighborhood offer both public terminals and free WiFi, or you could just enjoy the public WiFi on the steps of the Capitol Building!
contact
Northeast Branch Library
330 7th St NE
+1 202 698-3320
M,W 1PM-9PM; Tu,Th-Sa 9:30AM-5:30PM; Su 1PM-5PM
contact
Southeast Branch Library
403 7th St SE
+1 202 698-3377
M,W,Sa 9:30AM-5:30PM; Tu,Th 1PM-9PM; Su 1PM-5PM